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Organometallic Chemistry

Gordon Research Conference

Innovations in Ligand, Main Group and Metals as Platforms for Activation

July 7 - 12, 2019

Chair

Vice Chair

Salve Regina University

36 Ochre Point Avenue

Newport, Rhode Island, United States

Venue and Travel Information

Conference Description

Chemists are a vital part of the equation for solving many key scientific challenges. Society continues to rely heavily on the pioneering, comprehensive, and creative solutions from organometallic chemistry to solve scientific problems worldwide. The 2019 Organometallic Gordon Research Conference will afford the proper forum to temper initial innovative results from the collective insights of outstanding members of the field to advance promising new areas of scientific discovery. This seminal conference of organometallic chemistry is well attended by many esteemed research leaders working on the cutting edge of the field from academic, industrial, and government settings around the world. Comprised of a diverse array of established senior investigators, promising junior scientists, graduate students, and postdocs, this meeting serves as a focal point for organometallic chemistry. The newest directions and latest findings are presented, discussed, and evaluated. The professional forum created by the GRC fosters an atmosphere of inclusive, collaborative, and open discussion. Promising, yet primarily unpublished, results on vital innovations and novel compounds are shared with the goal of applying fundamental research to solve important problems. This conference will cover important themes shaping the organometallic landscape: ligand design, main group chemistry, transition metal catalysis, and many others. These topics have implications in organic/inorganic synthesis, polymerization, photochemistry, and small molecule activation.

All participants are strongly encouraged to support the conference objectives of full participation through attendance and the presentation of a poster highlighting recent work. Graduate students and postdoctoral fellows are also strongly encouraged to consider attending the Gordon Research Seminar (GRS) on Organometallic Chemistry (July 6-7, same location) that is geared toward promoting interaction and discussion among junior scientists.

Related Meeting

This GRC will be held in conjunction with the "Organometallic Chemistry" Gordon Research Seminar (GRS). Those interested in attending both meetings must submit an application for the GRS in addition to an application for the GRC. Refer to the associated GRS program page for more information.

Conference Program

Sunday
2:00 pm - 9:00 pm	Arrival and Check-in
6:00 pm - 7:00 pm	Dinner
7:30 pm - 7:40 pm	Introductory Comments by GRC Site Staff / Welcome from the GRC Chair
7:40 pm - 9:30 pm	Young Investigator Presentations Discussion Leader:
7:40 pm - 7:50 pm	Introduction by Discussion Leader
7:50 pm - 8:30 pm	"Mechanism of Ni-Catalyzed Alkene Functionalization and Applications in Stereoselective Synthesis"
8:30 pm - 8:40 pm	Discussion
8:40 pm - 9:20 pm	"Hydrocarbon Upgrading at Lattice-Confined Reactive Intermediates"
9:20 pm - 9:30 pm	Discussion
Monday
7:30 am - 8:30 am	Breakfast
9:00 am - 12:30 pm	Late Transition Metals Discussion Leader:
9:00 am - 9:30 am	"New Avenues in Late Transition Metal Carbene Chemistry"
9:30 am - 9:45 am	Discussion
9:45 am - 10:15 am	"Bond Activation and Catalytic Prospects with Boryl and Other Pincers"
10:15 am - 10:30 am	Discussion
10:30 am - 11:00 am	Coffee Break
11:00 am - 11:30 am	"Synthesis and Reactivity of a Terminal Co-Oxo Complex"
11:30 am - 11:45 am	Discussion
11:45 am - 12:15 pm	"New Breakthroughs in Catalytic Asymmetric Hydrogenation"
12:15 pm - 12:30 pm	Discussion
12:30 pm - 1:30 pm	Lunch
1:30 pm - 4:00 pm	Free Time
3:00 pm - 4:00 pm	The GRC Power Hour™ The GRC Power Hour™ is designed to address challenges women face in science and issues of diversity and inclusion. The program supports the professional growth of all members of our communities by providing an open forum for discussion and mentoring. Organizer:
4:00 pm - 6:00 pm	Poster Session
6:00 pm - 7:00 pm	Dinner
7:30 pm - 9:30 pm	Early or Earth Abundant First Row Transition Metals Discussion Leader:
7:30 pm - 8:00 pm	"Metalloradical Catalysis: Concept, Application and Mechanism"
8:00 pm - 8:10 pm	Discussion
8:10 pm - 8:40 pm	"Early Metals Do It Better but Some Exceptions May Apply: Taking Advantage of Metal-Carbon Multiple Bonds for the Transformative Chemistry of Hydrocarbons"
8:40 pm - 8:50 pm	Discussion
8:50 pm - 9:20 pm	"First-Row Transition Metal Complexes for the Electrocatalytic Reduction of CO₂, CO and O₂"
9:20 pm - 9:30 pm	Discussion
Tuesday
7:30 am - 8:30 am	Breakfast
8:30 am - 9:00 am	Group Photo
9:00 am - 12:30 pm	Cooperative Chemistry Utilizing Transition Metals Discussion Leader:
9:00 am - 9:30 am	"Beyond Active Sites: Bioinorganic Approaches to Molecular Electrocatalysis"
9:30 am - 9:45 am	Discussion
9:45 am - 10:15 am	"Targeting New Reactivity Using Main Group/Transition Metal Cooperative Chemistry"
10:15 am - 10:30 am	Discussion
10:30 am - 10:55 am	Coffee Break
10:55 am - 11:25 am	"Marrying Cationic Antimony Lewis Acids with Late Transition Metals: Impact on Electrophilic Catalysis"
11:25 am - 11:40 am	Discussion
11:40 am - 11:55 am	"Thermochemical and Kinetic Considerations for CO₂ Hydrogenation"
11:55 am - 12:05 pm	Discussion
12:05 pm - 12:20 pm	"Iridium-Promoted Conversion of Epoxides to Primary Alcohols Under Acidic Conditions Using Hydrogen"
12:20 pm - 12:30 pm	Discussion
12:30 pm - 1:30 pm	Lunch
1:30 pm - 4:00 pm	Free Time
4:00 pm - 6:00 pm	Poster Session
6:00 pm - 7:00 pm	Dinner
7:30 pm - 9:30 pm	Main Group Contributions Discussion Leader:
7:30 pm - 8:00 pm	"Boron Cluster Building Blocks and Reagents"
8:00 pm - 8:10 pm	Discussion
8:10 pm - 8:40 pm	"Main-Group Catalysts for Ring Opening Polymerization of Lactones"
8:40 pm - 8:50 pm	Discussion
8:50 pm - 9:20 pm	"Metal-Catalyzed Routes to Low-Valent Main Group Fragments"
9:20 pm - 9:30 pm	Discussion
Wednesday
7:30 am - 8:30 am	Breakfast
9:00 am - 12:30 pm	Industrial and Supported Catalysts Discussion Leader:
9:00 am - 9:30 am	"Ethylene Trimerization Using Chromium Pyridyl Amine Complexes: A Computational Study"
9:30 am - 9:45 am	Discussion
9:45 am - 10:15 am	"Rate and Selectivity Enhancements Achieved Through Ligand Design in Rhodium-Catalyzed Hydroformylation Reactions"
10:15 am - 10:30 am	Discussion
10:30 am - 10:55 am	Coffee Break
10:55 am - 11:25 am	"From the Lab to a Large-Scale Asymmetric Hydrogenation: The Menthol Process of BASF"
11:25 am - 11:40 am	Discussion
11:40 am - 11:55 am	"Mechanisms of Interfacial Ion-Coupled Electron Transfer at Graphite Conjugate Rhodium Complexes"
11:55 am - 12:05 pm	Discussion
12:05 pm - 12:20 pm	"Imidazolyl-Phenyl (IMP) Anions: A Modular Structure for Tuning Solubility and Coordinating Ability"
12:20 pm - 12:30 pm	Discussion
12:30 pm - 1:30 pm	Lunch
1:30 pm - 4:00 pm	Free Time
4:00 pm - 6:00 pm	Poster Session
6:00 pm - 7:00 pm	Dinner
7:00 pm - 7:30 pm	Business Meeting Nominations for the Next Vice Chair; Fill in Conference Evaluation Forms; Discuss Future Site and Scheduling Preferences; Election of the Next Vice Chair
7:30 pm - 9:30 pm	Photochemistry and Energy Technology Discussion Leader:
7:30 pm - 8:00 pm	"Red, Bright and Blue: Organometallic Design Strategies for Efficient Phosphorescence at the Edges of the Visible Spectrum"
8:00 pm - 8:10 pm	Discussion
8:10 pm - 8:40 pm	"Metal Chelate Complexes Enable High Voltage Aqueous Redox Flow Batteries"
8:40 pm - 8:50 pm	Discussion
8:50 pm - 9:20 pm	"Proton-Assisted Reduction of CO₂ by Cobalt Aminopyridine Macrocycles"
9:20 pm - 9:30 pm	Discussion
Thursday
7:30 am - 8:30 am	Breakfast
9:00 am - 12:30 pm	Ligand Architecture and Activity Discussion Leader:
9:00 am - 9:30 am	"Nucleophilic Pincer-NHC Group 9 Complexes in Catalysis"
9:30 am - 9:45 am	Discussion
9:45 am - 10:15 am	"Metalated Ylides: Powerful Reagents in Main Group Chemistry"
10:15 am - 10:30 am	Discussion
10:30 am - 10:55 am	Coffee Break
10:55 am - 11:25 am	"Manipulating the p-Block with d-Block Isocyanides"
11:25 am - 11:40 am	Discussion
11:40 am - 11:55 am	"Cyclobutadienyl Chemistry of the Rare-Earth Elements"
11:55 am - 12:05 pm	Discussion
12:05 pm - 12:20 pm	"Determining the Thermochemical Influence of Metal- Versus Ligand-Centered Protonation in Half Sandwich Complexes"
12:20 pm - 12:30 pm	Discussion
12:30 pm - 1:30 pm	Lunch
1:30 pm - 4:00 pm	Free Time
4:00 pm - 6:00 pm	Poster Session
6:00 pm - 7:00 pm	Dinner
7:30 pm - 9:30 pm	Keynote Session: Molecule Activation Discussion Leader:
7:30 pm - 8:10 pm	"Small Molecule Reduction Catalysis and a Role for Protonated Metallocenes"
8:10 pm - 8:25 pm	Discussion
8:25 pm - 9:05 pm	"Organometallic Electrocatalysis and the Reduction of CO₂"
9:05 pm - 9:20 pm	Discussion
9:20 pm - 9:30 pm	Closing Remarks
Friday
7:30 am - 8:30 am	Breakfast
9:00 am	Departure

Contributors

This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Acquisition & Assistance, under Award Number(s) DE-SC0019906. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof.

Support provided by Argonne National Laboratory.

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